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Ultrafast electron and material dynamics following femtosecond filamentation induced excitation of transparent solids

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Abstract

We examine the spatiotemporal dynamics of filamentation and subsequent material changes in two transparent media, fused silica and poly(methyl methacrylate) (PMMA), using inline holographic microscopy. We are able to dynamically observe the nonlinear propagation of femtosecond laser pulses and the consequent evolution of the electronic excitatio n and trapping inside the bulk of both materials. In the case of fused silica we reveal the physical conditions for the formation of nanogratings, measuring excited electron densities well below the critical density while for PMMA we show that excited electrons with densities exceeding 1018 cm−3, exhibit complex trapping dynamics in a 200 fs time scale. The clear demonstration of ultrafast sub-ps photochemical processes that take place during the irradiation of PMMA with femtosecond pulses will have a strong impact on the laser microprocessing of polymers and nanosurgery applications of bio-related materials.

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References

  1. R.R. Gattass, E. Mazur, Nat. Photon. 2, 219–225 (2008)

    Article  ADS  Google Scholar 

  2. L. Sudrie, A. Couairon, M. Franco, B. Lamouroux, B. Prade, S. Tzortzakis, A. Mysyrowicz, Phys. Rev. Lett. 89, 186601 (2002)

    Article  ADS  Google Scholar 

  3. S. Tzortzakis, L. Sudrie, M. Franco, B. Prade, A. Mysyrowicz, A. Couairon, L. Berge, Phys. Rev. Lett. 87, 213902 (2001)

    Article  ADS  Google Scholar 

  4. S.S. Mao, F. Quéré, S. Guizard, X. Mao, R.E. Russo, G. Petite, P. Martin, Appl. Phys. A Mater. Sci. Process. 79, 1695–1709 (2004)

    Article  ADS  Google Scholar 

  5. E.G. Gamaly, S. Juodkazis, K. Nishimura, H. Misawa, B. Luther-Davies, L. Hallo, P. Nicolai, V.T. Tikhonchuk, Phys. Rev. B 73, 214101 (2006)

    Article  ADS  Google Scholar 

  6. D.G. Papazoglou, S. Tzortzakis, Opt. Mater. Express 1, 625–632 (2011)

    Article  Google Scholar 

  7. A. Kaiser, B. Rethfeld, M. Vicanek, G. Simon, Phys. Rev. B 61, 11437–11450 (2000)

    Article  ADS  Google Scholar 

  8. P. Martin, S. Guizard, P. Daguzan, G. Petite, P. D’Oliveira, P. Meynadier, M. Perdrix, Phys. Rev. B 55, 5799–5810 (1997)

    Article  ADS  Google Scholar 

  9. D.G. Papazoglou, I. Zergioti, S. Tzortzakis, Opt. Lett. 32, 2055–2057 (2007)

    Article  ADS  Google Scholar 

  10. L. Sudrie, M. Franco, B. Prade, A. Mysyrowicz, Opt. Commun. 171, 279–284 (1999)

    Article  ADS  Google Scholar 

  11. E. Bricchi, B.G. Klappauf, P.G. Kazansky, Opt. Lett. 29, 119–121 (2004)

    Article  ADS  Google Scholar 

  12. Y. Shimotsuma, P.G. Kazansky, J. Qiu, K. Hirao, Phys. Rev. Lett. 91, 247405 (2003)

    Article  ADS  Google Scholar 

  13. C. Hnatovsky, R.S. Taylor, P.P. Rajeev, E. Simova, V.R. Bhardwaj, D.M. Rayner, P.B. Corkum, Appl. Phys. Lett. 87, 014104 (2005)

    Article  ADS  Google Scholar 

  14. V.R. Bhardwaj, E. Simova, P.P. Rajeev, C. Hnatovsky, R.S. Taylor, D.M. Rayner, P.B. Corkum, Phys. Rev. Lett. 96, 057404 (2006)

    Article  ADS  Google Scholar 

  15. W. Yang, E. Bricchi, P.G. Kazansky, J. Bovatsek, A.Y. Arai, Opt. Express 14, 10117–10124 (2006)

    Article  ADS  Google Scholar 

  16. J. Noack, A. Vogel, IEEE J Quantum Electron 35, 1156–1167 (1999)

    Article  ADS  Google Scholar 

  17. A. Vogel, J. Noack, G. Huttman, G. Paltauf, Appl. Phys. B 81, 1015–1047 (2005)

    Article  ADS  Google Scholar 

  18. B. Hopp, Z. Toth, K. Gal, A. Mechler, Z. Bor, S.D. Moustaizis, S. Georgiou, C. Fotakis, Appl. Phys. Mater. Sci. Process. 69, S191–S194 (1999)

    ADS  Google Scholar 

  19. F. Beinhorn, J. Ihlemann, K. Luther, J. Troe, Appl. Phys. A 79, 869–873 (2004)

    Article  ADS  Google Scholar 

  20. S. Sowa, W. Watanabe, J. Nishii, K. Itoh, Appl. Phys. A 81, 1587–1590 (2005)

    Article  ADS  Google Scholar 

  21. D. Gomez, I. Goenaga, I. Lizuain, M. Ozaita, OptEn 44, 051105 (2005)

    ADS  Google Scholar 

  22. G. Zhou, M. Ventura, M. Gu, A. Matthews, Y. Kivshar, Opt. Express 13, 4390–4395 (2005)

    Article  ADS  Google Scholar 

  23. C. Schaffer, N. Nishimura, E. Glezer, A. Kim, E. Mazur, Opt. Express 10, 196–203 (2002)

    Article  ADS  Google Scholar 

  24. C.L. Thomsen, D. Madsen, S.R. Keiding, J. Thogersen, O. Christiansen, JChPh 110, 3453–3462 (1999)

    ADS  Google Scholar 

  25. S. Minardi, A. Gopal, M. Tatarakis, A. Couairon, G. Tamosauskas, R. Piskarskas, A. Dubietis, P. Di Trapani, Opt. Lett. 33, 86–88 (2008)

    Article  ADS  Google Scholar 

  26. G. Zhang, J.K. Thomas, J. Phys. Chem. A 102, 5465–5475 (1998)

    Article  Google Scholar 

  27. C.L. Arnold, A. Heisterkamp, W. Ertmer, H. Lubatschowski, Appl. Phys. B 80, 247–253 (2005)

    Article  ADS  Google Scholar 

  28. C.L. Arnold, A. Heisterkamp, W. Ertmer, H. Lubatschowski, Opt. Express 15, 10303–10317 (2007)

    Article  ADS  Google Scholar 

  29. M. Szadkowska-Nicze, J. Mayer, J. Polym. Sci. Part A Polym. Chem. 36, 1209–1215 (1998)

    Article  ADS  Google Scholar 

  30. A. Baum, P.J. Scully, M. Basanta, C.L.P. Thomas, P.R. Fielden, N.J. Goddard, W. Perrie, P.R. Chalker, Opt. Lett. 32, 190–192 (2007)

    Article  ADS  Google Scholar 

  31. A. Baum, P.J. Scully, W. Perrie, D. Jones, R. Issac, D.A. Jaroszynski, Opt. Lett. 33, 651–653 (2008)

    Article  ADS  Google Scholar 

  32. D.G. Papazoglou, S. Tzortzakis, Appl. Phys. Lett. 93, 041120 (2008)

    Article  ADS  Google Scholar 

  33. D. Abdollahpour, D.G. Papazoglou, S. Tzortzakis, Phys. Rev. A 84, 053809 (2011)

    Article  ADS  Google Scholar 

  34. A. Couairon, A. Mysyrowicz, Phys. Rep. 441, 47–189 (2007)

    Article  ADS  Google Scholar 

  35. P.P. Rajeev, M. Gertsvolf, E. Simova, C. Hnatovsky, R.S. Taylor, V.R. Bhardwaj, D.M. Rayner, P.B. Corkum, Phys. Rev. Lett. 97, 253001 (2006)

    Article  ADS  Google Scholar 

  36. E. Hauge, S.A. Naroo, W.N. Charman, J. Cataract Refract. Surg. 27, 2026–2035 (2001)

    Article  Google Scholar 

  37. B.C. Stuart, M.D. Feit, S. Herman, A.M. Rubenchik, B.W. Shore, M.D. Perry, Phys. Rev. B 53, 1749 (1996)

    Article  ADS  Google Scholar 

  38. K.R. Siefermann, B. Abel, Angewandte Chemie Int Edition 50, 5264–5272 (2011)

    Article  Google Scholar 

  39. D.E. Hare, D.D. Dlott, Appl. Phys. Lett. 64, 715–717 (1994)

    Article  ADS  Google Scholar 

  40. S. Kuper, S. Modaressi, M. Stuke, J. Phys. Chem. 94, 7514–7518 (1990)

    Article  Google Scholar 

  41. T. Mitsuoka, A. Torikai, K. Fueki, J. Appl. Polym. Sci. 47, 1027–1032 (1993)

    Article  Google Scholar 

  42. L.M. Barker, R.E. Hollenbach, J. Appl. Phys. 41, 4208–4226 (1970)

    Article  ADS  Google Scholar 

  43. R.M. Waxler, D. Horowitz, A. Feldman, Appl. Opt. 18, 101–104 (1979)

    Article  ADS  Google Scholar 

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Acknowledgments

We gratefully acknowledge the inspiration and impact in this work of the late Savas Georgiou, to whose memory we dedicate this article. We also wish to acknowledge helpful discussions with Nikita Bityurin. This work was supported by the European Union Marie Curie Excellence Grant “MULTIRAD” MEXT-CT-2006-042683 and in part by the EU FP7 Programs “LASERLAB-EUROPE” I and II.

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Authors and Affiliations

  1. Institute of Electronic Structure and Laser, Foundation for Research and Technology Hellas, P.O. Box 1527, 71110, Heraklion, Greece

    Dimitrios G. Papazoglou, Daryoush Abdollahpour & Stelios Tzortzakis

  2. Materials Science and Technology Department, University of Crete, P.O. Box 2208, 71003, Heraklion, Greece

    Dimitrios G. Papazoglou & Stelios Tzortzakis

Authors
  1. Dimitrios G. Papazoglou
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  2. Daryoush Abdollahpour
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  3. Stelios Tzortzakis
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Correspondence to Dimitrios G. Papazoglou or Stelios Tzortzakis.

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Papazoglou, D.G., Abdollahpour, D. & Tzortzakis, S. Ultrafast electron and material dynamics following femtosecond filamentation induced excitation of transparent solids. Appl. Phys. A 114, 161–168 (2014). https://doi.org/10.1007/s00339-013-8114-4

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  • DOI: https://doi.org/10.1007/s00339-013-8114-4

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