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Application of LIF to investigate gas transfer near the air-water interface in a grid-stirred tank

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Abstract

The interaction between oxygen absorption into liquids and bottom shear-induced turbulence was investigated in a grid-stirred tank using a laser-induced fluorescence (LIF) technique. The LIF technique enabled visualization as well as quantification of planar concentration fields of the dissolved oxygen (DO) near the air-water interface. Qualitative observation of the images provided more insight into the physical mechanism controlling the gas transfer process. The high data resolution is an advantage for revealing the concentration distribution within the boundary layer, which is a few hundreds of a micrometer thick. Mean and turbulent fluctuation characteristics were obtained and compared with previous results.

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References

  • Atmane MA, George J (2002) Gas transfer across a zero-shear surface: a local approach. Geophys Monogr 127, Gas Transfer at Water Surfaces, pp 255–259

  • Brumley BH, Jirka GH (1987) Near-surface turbulence in a grid-stirred tank. J Fluid Mech 183:236–263

    Google Scholar 

  • Brutsaert WH, Jirka GH (1984) Gas transfer at water surfaces. D. Reidel Publishing Co

  • Chu CR, Jirka GH (1992) Turbulent gas flux measurements below the air-water interface of a grid-stirred tank. Int J Heat Mass Transfer 35(8):1957–1968

    Article  CAS  Google Scholar 

  • Churchill M (1961) Effect of water temperature on stream reaeration. J Sanitary Eng Div 5(87):59–71

    Google Scholar 

  • Danckwerts PV (1951) Significance of liquid-film coefficients in gas absorption. Indust Eng Chem 43:1460–1467

    CAS  Google Scholar 

  • Duke SR, Hanratty TJ (1995) Measurement of the concentration field resulting from oxygen absorption at a wavy air-water interface. Air-Water Gas Transfer: 3rd Int Symp on Air-Water Gas Transfer, pp 627–635

  • Fortescue GE, Pearson JR (1967) On gas absorption into a turbulent liquid. Chem Eng Sci 22:187–216

    Google Scholar 

  • Higbie R (1935) The rate of absorption of a pure gas into a still liquid during short periods of exposure. AIChE Trans 31:365–390

    CAS  Google Scholar 

  • Hopfinger EJ, Toly JA (1976) Spatially decaying turbulence and its relation to mixing across density interfaces. J Fluid Mech 78:155–175

    Google Scholar 

  • Jähne B, Haussecker H (1998) Air-water gas exchange. Annu Rev Fluid Mech 30:443–468

    Article  Google Scholar 

  • Lamont JC, Scott DS (1970) An eddy cell model of mass transfer into the surface of a turbulent liquid. AIChE J 16:513–519

    CAS  Google Scholar 

  • Lee M (2002) Visualization of oxygen transfer across the air-water interface using a fluorescence oxygen visualization method. Water Res 36:2140–2146

    Article  CAS  PubMed  Google Scholar 

  • Lee Y (1977) Microprobe method for studying gas-liquid oxygen transfer in various surfactant systems. PhD Thesis, Purdue University

  • Lewis WK, Whitman W (1924) Principles of gas absorption. Ind Eng Chem 16

  • Münsterer T, Jähne B (1998) LIF measurement of concentration profiles in the aqueous mass boundary layer. Exp Fluids 25:190–196

    Article  Google Scholar 

  • Münsterer T, Mayer H, Jähne B (1995) Dual-tracer measurements of concentration profiles in the aqueous mass boundary layer. Air-Water Gas Transfer: 3rd Int Symp on Air-Water Gas Transfer, pp 637–648. Application of LIF to investigate gas transfer 21

  • Schladow S, Lee M, Hrzeler B, Kelly P (2002) Oxygen transfer across the airwater interface by natural convection in lakes. Limnol Oceanogr 47(5):1394–1404

    CAS  Google Scholar 

  • Thompson SM, Turner JS (1975) Mixing across an interface due to turbulence generated by an oscillating grid. J Fluid Mech 67:349–368

    Google Scholar 

  • Vaughan WM, Weber G (1970) Oxygen quenching of pyrenebutyric acid fluorescence in water, a dynamic probe of the microenvironment. Biochemistry 9:464–473

    CAS  PubMed  Google Scholar 

  • Wolff LM, Hanratty TJ (1994) Instantaneous concentration profiles of oxygen accompanying absorption in a stratified flow. Exp Fluids 16:385–392

    CAS  Google Scholar 

  • Wolff LM, Liu ZC, Hanratty TJ (1990) A fluorescence technique to measure concentration gradients near an interface. Proc 2nd Int Symp on Gas Transfer at Water Surfaces, pp 210–218

  • Woodrow PT, Duke SR (2001) Laser-induced fluorescence studies of oxygen transfer across unsheared flat and wavy air-water interfaces. Ind Eng Chem Res 40:1985–1995

    Article  CAS  Google Scholar 

Download references

Acknowledgements

This project was funded by the “German Science Foundation” (DFG Grant No. Ji18/7–1). The authors would like to express their appreciation for the constructive suggestions from anonymous reviewers.

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Correspondence to Herlina or G. H. Jirka.

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Herlina, Jirka, G.H. Application of LIF to investigate gas transfer near the air-water interface in a grid-stirred tank. Exp Fluids 37, 341–349 (2004). https://doi.org/10.1007/s00348-004-0822-2

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  • DOI: https://doi.org/10.1007/s00348-004-0822-2

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