Introduction

Back-n is a white neutron source associated with the CSNS high energy proton accelerator, which has been running since 2018. The main motivation of this facility is for the nuclear data measurement and neutron detector calibration. More than hundreds experiments have been accomplished since the beginning of the operation, including \(^{235}\)U/\(^{238}\)U fission cross section measurement [1], neutron induced light charged particle emission cross section measurement of \(^{6}\)Li and \(^{10}\)B [2, 3], and others. Some of the results were collected by the EXFOR (Experimental Nuclear Reaction Data) [4] and evaluated by consultants on Neutron Data Standards [5].

Fig. 1
figure 1

The layout of the back-n beamline and the detectors’ location

Figure 1 shows the layout of the Back-n beamline and detectors’ locations. The 1.6 GeV proton beam hits the tungsten target with a 15\(^{\circ }\) deflection. The back-streaming neutrons are leading to the Back-n tunnel, which has a long flight distance for the neutron time-of-flight method. Two end stations ES#1 and ES#2 are constructed for different nuclear data measurements. The ES#1 has a distance of about 55 m, and ES#2 is about 70 m from the target.

The beam diagnostics and several detector systems, for example the Fission chamber, the light charged particle detector array, the C\(_{6}\)D\(_{6}\) scintillation detectors and the camera system were developed before the beamline established and serviced most of the experiments at Back-n. Several ambitious developments, for example, the multi-purpose time projection chamber (MTPC) , the radiation resistant semiconductor detectors, the Gamma-ray total absorption facility (GTAF-II) and the neutron-sensitive micro-channel-plate detector (B-MCP) are in progress for future experiments. The layout of the Back-n beamline and the locations of the detectors can be found in Fig. 1.

This article follows the classification of detectors, which can be divided into beam diagnostic systems, detector systems for different particles, and neutron resonance radiography systems. It also includes the electronics and DAQ systems used by these detectors.

Detectors for neutron beam characterization and monitoring

Beam diagnostics is basic component for the beamline construction and running. Back-n has built an online flux monitor (Li-Si detector), a neutron energy measurement detector (Fission chamber) and a beam profile detector (Micromegas).

Li–Si beam flux monitor

A \({}^{6}\textrm{Li}\)F-silicon detector array was developed for real-time neutron monitoring at the back-n white neutron beam. It is installed on the beamline and works simultaneously with the nuclear data measurements to provide neutron flux data for normalization of the experiments [6].

To minimize beamline interference and background, the monitor was designed as a structure with a \({}^{6}\textrm{Li}\)F neutron conversion layer and Si detector array separated. \({}^{6}\textrm{Li}\)F is deposited on a 10 \(~\upmu \)m Al film with a thickness of 360 \(~\upmu \)g/cm\({}^2\) and placed on the beamline with an area of \(~\phi \) 80 mm covering the maximum beam envelope. Eight identical Si detectors are placed symmetrically on the side of the \({}^{6}\textrm{Li}\)F layer and upstream of the beam to reduce scattered neutron background. The sensitive area center of the Si detectors is on the diagonal of the beamline and the layer center. The bottom edge of the Si detector is outside the beam envelope to avoid direct irradiation by the neutrons. The monitor is shown in Fig. 2. It is entirely installed in the middle of a vacuum tube with a length of 40 cm and flanged to the other vacuum tubes on the beamline. Two Li-Si monitors were mounted in ES#1 and ES#2, and the distance between the \({}^{6}\textrm{Li}\)F layer and the tungsten target is 54.36 m and 73.76 m, respectively. A RF60 flange with nine vacuum-tight Lemo connectors is on the side of the tube. Electronic signals from the Si detectors are taken out through the connectors and connected to the input of MSI-8, a multi-function amplifier from Mesytec [7]. The voltage on the Si detector is -30 V and is supplied by a custom power supply, which was designed to supply voltages to both the Si and MSI-8 preamplifier.

Fig. 2
figure 2

Pictures of the Li–Si monitor

The well-known cross section for the \({}^{6}\textrm{Li} (n,\,t) {}^{4}\textrm{He}\) reaction allows to monitor the neutron flux from thermal to approximately 1 MeV energies [8]. The reaction products \(~\alpha \) and \(^{3}\)H are emitted opposite to each other according to the principle of momentum conservation, which ensures that the Si detectors do not have double counting. The monitor count rate reflects the neutron fluence rate, which is consistent with the proton power on the target. The conversion factor requires a calibration using \(^{235}\)U/\(^{238}\)U fission chamber, which gives measurement of the actual neutron fluence rate. Good performance was obtained when the Li-Si monitor was mounted on the beamline for monitoring experiments. Figure 3 shows the real-time online results obtained by the Li-Si monitor when CSNS operates at a frequency of 25 Hz and proton beam power of 100 kW. The (a) is a typical waveform of a neutron signal, and (b) is the integral spectrum of the signal pulse height, in which the peak of \(~\alpha \)-particles and tritons can be clearly identified. The (c) shows the online curve of count rate. Few downward spikes in the figure may be caused by the instantaneous drop of the beam power due to a flash fire or other reasons. Although the curve has a large fluctuation with the measuring time in figure (c), it has good stability after being normalized to the beam power. As shown in (d), the counting rate is approximately 45.28 per 10 kW and the uncertainty is less than 1\(\%\), which includes statistical and systematic errors. The insert shows that there is a stable conversion factor between the proton flux and the monitor counts over a long period of time. In general, the calibrated monitor counts and integral protons can equivalently reflect the neutron flux during the monitoring period. In the case of stable energy spectrum of Back-n, the entire neutron flux can be obtained by a conversion factor and without having to detect neutron events over all the energy regions.

Fig. 3
figure 3

a A typical waveform of a neutron signal; b the integral spectrum of the signal pulse height; c the online count rate curve of the monitor; d The monitor counts per second at 10 kW proton beam power. Comparison of the counts and proton flux in time stages is shown in insert [6]

The cross section of \(^{6}\)Li is very smooth and accurate in the neutron energy below 1 MeV. The detailed structure of the energy spectrum can be well measured by the monitor especially in the energy region below 10 keV, which are difficult to be analyzed by fission chamber with \(^{235}\)U target, since the \(^{235}\)U target has many resonances in the neutron cross section in this region [9]. The neutron energy is determined by the TOF method which defines the neutron velocity as \(V=L/T\), where L is the flight path from the tungsten target to the \(^{6}\)LiF layer and the T is the time-of-flight of neutrons obtained by the time interval between the time recorded by the detector and the trigger T\(_{0}\). For the neutrons below 10 keV, the effect of the \(\Delta {T}\) is much less than 1\(\%\), and the \(\Delta {L}\) can be calibrated by comparing the energy spectrum detail structure of the hyperthermal neutrons (1–10 eV) to that measured by the \(^{235}\)U fission chamber. With determined L and T, the kinetic energy of neutrons can be calculated with the relativity formula. The neutron spectrum is obtained by dividing the counting rate by the cross sections of \(^{6}\)Li extracted from ENDF-B/VIII.0 [10]. The result is normalized to 100 kW beam power and is shown together with the spectrum measured by the \(^{235}\)U fission chamber with 100 bpd, as shown in Fig. 4 [11]. The energy spectrum below 10 keV measured by the monitor agrees with the spectrum measured by the \(^{235}\)U target pretty well in the overall trend and without the resonance peaks. We compared the details of the two spectra in the energy region of 2.5–5 keV. As shown in the insert, the details of the two spectra outside of the resonance region can basically coincide.

Fig. 4
figure 4

The comparison of the neutron energy spectrum measured by the Li–Si monitor and the \(^{235}\)U fission chamber. The detailed structure of 2.5–5 keV region is in the insert [6]

Fission ionization chamber for neutron energy spectrum measurement

The fission chamber is dedicated to measuring neutron energy spectrum of Back-n, which is composed of several targets, electrodes, shielding, insulating parts, signal wires, inlet and outlet feedthroughs, etc., as shown in Fig. 5. The fission chamber adopts a copper shielding chamber and electrodes. The target substrate is a platinum plate with a thickness of 0.2 mm and a diameter of 32 mm. The diameter of the active area of the target is 20 mm. The total amount of the enriched uranium coating is 832.97 \(~\upmu \)g . The collection electrode, the target plate and the chamber are separated by insulating materials, and the distance between the target plate and the collector is controlled by the varying thickness of the insulating gasket. The target is grounded, and the collector is connected to the ORTEC-142B preamplifier, which is connected to a positive high voltage of 400 V. The fission chamber adopts a gas flow design, and the working gas is argon-methane P10 (10\(\%\) methane, 90\(\%\) argon).

Fig. 5
figure 5

Schematic diagram of the fission chamber for testing

The ability to distinguish noise and fission signals is obtained by adjusting parameters such as electrode spacing and voltage, in Fig. 6. The experimental results show that when the distance between the electrodes is small, the energy spectrum of the fission chamber is generally lower. The \(\alpha \) decay events and fission events are mixed together; with the increase in the distance between the plates, the fission fragment peak and the \(\alpha \) peak are gradually distinguished, and the peak-to-valley ratio of the fission fragment is getting higher; when the distance reaches 10 mm, the identification between the fission fragment and the \(\alpha \) particle can be counted more accurately.

Fig. 6
figure 6

Energy spectrum of \(^{235}\)U fission chamber with different plate spacing

Using the 14 MeV pulsed neutron beam generated by the D-T fusion reaction at the 600 kV Cockcroft-Walton generator of the China Institute of Atom Energy, the time correlation spectrum between the output signal of the fission chamber and the pick-up signal was measured, while the plate spacing was 10 mm, as shown in Fig. 7. The distance between the fission chamber and the tritium target head is 1.5 cm, and the neutron flight time is about 0.28 ns, which can be ignored. The rise time of the output signal of the fission chamber model was measured to be about 30 ns using an oscilloscope. With a Gaussian fitting, the FWHM of the fission signal peak is 30.97 channels in TAC, and the time resolution calculated according to the TAC channel width is 14.7 ns. The time resolution mainly comes from two contributions, the pulse width of the pulse beam and the time resolution of the detector. The pulse beam width is 2–3 ns, and the contribution to the time resolution is very small, so it can be considered that the measured time resolution is the detection time resolution of the device.

Fig. 7
figure 7

Temporal correlation spectrum between the output signal of the \(^{235}\)U fission chamber and the pick-up signal

The fission reaction generally produces two fission fragments with opposite directions. When the direction is parallel to the target surface, both fragments cannot be detected. Therefore, the detection efficiency of the fission chamber is shown in Eq. 1, which is related to the number of target nuclei N , the fission cross section of \(\sigma _{f}\)(E), and the detection efficiency \(\varepsilon _{f}\) of fission fragments, where \(\varepsilon _{f}\) is less than 100 \(\%\) . The neutron flux \(\phi \) can be deduced by the companion particle method, and the detection efficiency of the fission chamber can also be obtained in combination with the fission chamber count rate N\(_{f}\).

$$\begin{aligned} \varepsilon \left( E \right) =\frac{N_{t} }{\phi } =N\cdot \sigma _{f} \left( E\right) \cdot \varepsilon _{f} \end{aligned}$$
(1)

As a result of calibration, with the 14 MeV neutron test, the detection efficiency is 4.3\(\times 10^{-6}\) , and the uncertainty is less than 5\(\%\). The final Back-n neutron energy spectrum measured by this calibrated fission chamber can be found in reference [11].

Fig. 8
figure 8

Micromegas fabrication process. a The mesh after thermocompression bonding. An array of cylindrical pillars is visible, which hold the mesh and ensure a constant distance between the mesh and the PCB. b The detector chamber

Micromegas for neutron beam profile measurement

Measurement of the neutron beam spot distribution is the basic requirement for the Back-n facility. Thanks to the good two-dimensional (2D) spatial resolution and fast timing capability of the Micromegas (micro-mesh gaseous structure) detector [12, 13], it can be used for a quasi-online measurement of the neutron beam profile, e.g., at the n_TOF facility [14] and at the Back-n white neutron facility [15].

Micromegas detectors (MDs) have been widely used in nuclear and particle physics including rare event searches [16, 17] and neutron detection [18]. In this section, we present the development of an MD with 2D spatial resolution capability for the measurement of the neutron beam spot distribution. The current setup of the MD, used as a beam profiler at Back-n, sums up the neutron events of the entire energy range, with higher weights on low-energy neutrons due to higher cross sections \({}^{10}\textrm{B} (n,\,\alpha ) {}^{7}\textrm{Li}\) and \({}^{6}\textrm{Li} (n,\,t) {}^{4}\textrm{He}\). However, it is planned, as part of the future detector development, to improve the MD system design so as to obtain the energy dependence of the neutron beam profile of Back-n.

Figure 8 shows the MD of this work. A thin layer of \({}^{10}\textrm{B}\) or \({}^{6}\textrm{Li}\) deposited on a thin aluminum foil is used as the neutron converter. The neutron converter is attached to the cathode electrode facing the drift gap (i.e., the region between cathode and mesh). The mesh-anode avalanche gap (an amplification region where electron avalanches occur) is manufactured with the thermal bonding method (see Ref. [19] for detailed description of the manufacturing process). With this method, each side of the readout PCB is attached to a metallic mesh to form the avalanche gap, and a back-to-back structure is obtained (see Fig. 9). These two avalanche structures are able to work simultaneously for a higher detection efficiency. The avalanche gap and the drift gap are 100 \(\upmu \)m and 5 mm, respectively. The total active area of the MD is 90 mm \(\times \) 90 mm. The layout and description of the MD are described in detail in Ref. [15].

Fig. 9
figure 9

Schematic of the MD with back-to-back double-avalanche structure. The mesh (dashed line) separates the 5 mm drift gap from the 100 \(\upmu \)m avalanche gap. Each of the XY readout strips is independently connected to the central board

Two detector units (namely MD-MA and MD-RA) with different anode designs are fabricated and characterized with a \({}^{55}\textrm{Fe}\) X-ray source to obtain the relative electron transparency, the gain and the gain uniformity, and the energy resolution [15]. For MD-MA, copper anode is used; for MD-RA, resistive anode with germanium coating is used. The resistive layer protects the detector from discharges caused by possible intense ionization. Although the resistive anode MD-RA is relatively more complex to fabricate than the copper anode MD-MA, the former has higher gain than the latter. A dedicated front-end electronics system based on the AGET ASIC chip [20, 21] is developed to process the anode strip signals [22]. In total, two AGET chips with 128 channels are used. The signal is amplified by a charge sensitive preamplifier and a shaping amplifier, and subsequently digitized by a multi-channel analyzer.

The neutron beam profile reconstruction capability of the detectors has been tested with an \({}^{241}\textrm{Am}\) \(\alpha \) source, an Am-Be neutron source, and the CSNS Back-n neutron beam (Fig. 10). Figure 11 shows the 2D neutron beam profile at the Back-n ES\(\#\)1 measured by the MD-MA with \({}^{10}\textrm{B}\) converter. The good agreement between the simulation and experimental data confirms the reliability of this measurement, as shown in Fig. 12 [15].

Fig. 10
figure 10

The MD together with the front-end electronics system was placed in the shielding container made of aluminum, as a neutron beam profiler at Back-n ES#1. The arrows represent the incoming neutron beam

Fig. 11
figure 11

The reconstructed 2D profile of the Back-n white neutron beam at ES#1. The bin widths for the 2D histogram are 1.5 mm on both the horizontal and vertical axes. The shaded dots in the profile image correspond to the reconstructed positions of the insulating pillars between the mesh and the anode plane

Fig. 12
figure 12

The upper panels show the 1D projections of the slices of the 2D profile corresponding to a the middle Y-strip onto the X-axis and b the middle X-strip onto the Y-axis, for both data (solid squares) and MC simulation (solid curves). The expectation from MC simulation is normalized to data. The lower panels contain the significance of the deviation between the observed data and the simulation prediction in each bin of the distribution, considering only the statistical fluctuations in data

Detectors for measuring fission cross sections and light charged particle emissions

Back-n used a fast fission ionization chamber to measure fission fragments and an light charged particle detector array to measure light charged particles. In future experiments, fragmentation fragments and light charged particles tend to use the same kind of detector system. So a multi-purpose time projection chamber and next generation semiconductor detectors have been developed as an option.

Multilayer fission ionization chamber

The fission ionization chamber as a reliable approach has been used for neutron induced fission cross section measurements for many years [23, 24]. A multi-cell fast fission ionization chamber (FIC) has been developed as an initial detector for Fast Ionization Chamber Spectrometer for Fission Cross Section Measurement (FIXM) at Back-n [25, 26]. FIXM contains FIC, front-end electronics, data acquisition (DAQ) system and peripheral supporting system and is mounted at the ES#2 as shown in Fig. 13.

FIC with an aluminum shell of \(\phi \)300 mm \(\times \) 300 mm and 5 mm thick is filled with a gas mixture of 90\(\%\) Ar and 10\(\%\) CF\(_{4}\) at a pressure of 800 mbar. The two neutron beam windows of \(\phi \)80 mm are sealed with 100-\(\upmu \)m-thick Kapton films and located in the center of the fission chamber caps. There are eight independent cells including seven cells with high-purity fissile materials enriched over 99.94\(\%\) and one blank cell inside the fission chamber and mounted along the direction of the neutron beam. Each cell consists of two electrodes of \(\phi \)80 mm with a gap of 5 mm, in which the fission fragments produced by fission reaction ionize the gas to generate signals. The gap, the capacitance and the high voltage of +200 V between electrodes are optimized in order to provide electrons having enough drift velocity, which is beneficial to obtain fast signals for high timing precision. A stainless steel of 20 \(\upmu \)m thickness or aluminum foil of 100 \(\upmu \)m thickness electroplated with the fissile material is the cathode, while the anode is made of aluminum foil of 100 \(\upmu \)m thickness. The diameter of about 50 mm and uniformity of the fission coating are measured by the alpha-sensitive imaging method, and its mass is determined with the \(\alpha \)-particle spectra measured in a small solid angle device  [27]. The aluminum anode collects ionization signals by connecting to an 8-channel preamplifier MSI-8 in which the gain of each channel can be independently adjusted. The output signals of MSI-8 are entered in the common DAQ in which the signals are conditioned, digitized and stored. After several upgrades and performance tests at neutron sources, the improved FIC has a reliable and stable performance with the rise time of fission fragment signals of less than 30 ns from 10 to 90\(\%\) and a high signal-to-noise ratio. The \({^{236,238}}\)U/\({^{235}}\)U fission cross section ratios from threshold energy to tens MeV were measured by using FIC and time-of-flight method at Back-n, and the results verify the reliability of FIC  [1, 28]. FIXM could be used to measure fission cross sections of various isotopes covering a wide neutron energy region.

Fig. 13
figure 13

Photograph of FIXM in Back-n beamline

Light charged particle detector array

In cross section measurements of neutron induced light charged particles emission (nlcp) reactions, detection and identification of charged particles are essential. Detection setups comprised of detectors, for example, grid ionization chambers, silicon detectors and scintillators, are usually adopted in previous measurements [29,30,31,32,33]. Based on these detection setups, particle identification(PID) of charged particles is realized with method such as \(\Delta {E}\)-E method.

At Back-n, a light charged particle detection array(LPDA) has been built and applied to experiments. Sixteen units \(\Delta {E}\)-\(\Delta {E}\)-E telescopes are placed in a vacuum chamber with a diameter of 1 m. Each telescope is composed of a low-pressure multi-wire proportional chamber(LPMWPC) [34, 35], a 2.5 cm\(\times \)2.5 cm PIN silicon detector and a cube CsI(Tl) detector with a side length of 3 cm. Thickness of each silicon detector is 300\(~\upmu \)m. The angle between two adjacent telescopes is 9.5 degree. As Fig. 14 illustrates, with eight telescopes sealed in one cavity, the telescopes are divided into two identical parts. The entrance window of the cavity is replaceable, and a 4\(~\upmu \)m polypropylene foil is used as an entrance window in default. The distances between the surface of the LPMWPC, silicon detector and CsI(Tl) detector are 205, 214 and 222 mm, respectively. LPMWPCs and silicon detectors are connected to charge-sensitive preamplifiers that are mounted behind CsI(Tl) detectors in the cavity. Besides, optical signals produced in a CsI(Tl) detector are collected and converted to electric signal by a 2.1 cm\(\times \)2.1 cm SiPM. During an experiment, the cavity will be filled with the working gas of the LPMWPC, usually 0.2 atm Ar+CO\(_{2}\), which means that all detectors and charge sensitive preamplifiers in the cavity also work under the gas environment. To stable the pressure in the cavity, an air pressure control system is applied to ensure that the pressure in the cavity is ±200 Pa near the preset value. Besides, as Fig. 14 shows, a target holder on which four targets can be mounted is installed on the target chamber cover, and the center of different targets can be moved from top to bottom to the beam center position with the movement of the remote control motor.

Fig. 14
figure 14

Photo of LPDA at Back-n. Sixteen telescopes are divided into two identical parts; the target holder is at the center of the vacuum chamber

In each telescope, the LPMWPC is used to identify the low-energy particles, and the CsI(Tl) detectors are applied to particles with higher energy. Results of an in-beam test indicate that using the \(\Delta {E}\)-E method, protons in the energy range of 0.5 MeV to 100 MeV can be identified by the telescope [34]. Besides the \(\Delta {E}\)-E method that two detectors required, the amplitude-\(E_\mathrm{{n}}\) method and pulse shape discrimination method are also adopted to identified particles using silicon detectors [36]. In the amplitude-\(E_\mathrm{{n}}\) method, \(E_\mathrm{{n}}\) is deduced from the measured time-of-flight information. The amplitude-\(E_\mathrm{{n}}\) method is utilized in \(\mathrm {^{10}B}(n,\alpha )\mathrm {^7Li}\) and \(\mathrm {^6Li}(n,t)\mathrm {^4He}\) cross section measurement reactions. Simultaneously, the pulse shape discrimination of silicon detectors is achieved with a charge and current sensitive preamplifier. The detector combination and PID method depend on the goal and emission particles’ energy.

As part of the LPDA, a silicon detector array and \(\Delta {E}\)-E telescopes have been applied to several experiments. Cross sections of \(\mathrm {^{10}B}(n,\alpha )\mathrm {^7Li}\), \(\mathrm {^6Li}(n,t)\mathrm {^4He}\), \(\mathrm {^1H}\) \((n,n)\) \(\mathrm {^1H}\) and \(\mathrm {^2H}\) \((n,n)\) \(\mathrm {^2H}\) reactions have been measured and published [3, 37, 38].

Multi-purpose time projection chamber

As a kind of detector with excellent three-dimensional tracking capability for measurements of particle momentum, spatial position, angular distribution and particle identification, time projection chambers (TPCs) have been widely used in particle and nuclear physics [39]. In recent years, TPC has also been adopted to the research of neutron nuclear data measurement [40], providing a new powerful tool for the cross sections of difficult measured with traditional methods.

To meet the requirements of nuclear data measurement, a multi-purpose time projection chamber (MTPC) is proposed at Back-n mainly for the light charged particle emission reaction, at the same time, other kinds of measurement such as fission reaction, neutron beam profile and neutron imaging can also be carried out with the MTPC.

A MTPC has been built and tested at Back-n. The schematic is shown in Fig. 15. The MTPC has a cylindrical sensitive volume of diameter of 140 mm. To form a uniform drift electric field, a height adjustable field cage shown in Fig. 16 composed of stacked PCB rings is designed to meet different measurements requirements. The readout anode PCB is connected at the end of the field cage. At the center of the anode PCB (Fig. 17), an array of 1519 hexagonal pads is fabricated to collect the deposited charge. A resistive Micromegas structure [19] is stretched on the surface of the anode PCB for the purpose of ionization electron avalanche as shown in Fig. 18. With the coating of the high-resistance germanium film layer on the anode surface, the high-voltage stability of the detector is obviously improved and a higher spatial resolution is obtained due to the effect of charge dispersion on the resistive layer [41].

Fig. 15
figure 15

The schematics of the MTPC structure

Fig. 16
figure 16

The field cage of MTPC

Fig. 17
figure 17

The anode PCB of MTPC

Fig. 18
figure 18

The structure of micromegas

The structure of the electronics system of the MTPC is shown in Fig. 19. The introduction of the electronics system in details can be found in Ref. [42] and a brief introduction is given here. At the front-end of the system are the pre-amplifier module (PAM), the analog-to-digital module and the power clock management module (PCMM), and the back-end is composed of the data concentration module (DCM) and trigger clock module (TCM). The main parameters of the electronics system are listed in Table. 1.

Fig. 19
figure 19

The structure of electronics system

Table 1 Key parameters of the electronics system

The MTPC has been commissioned with the white neutron beam at Back-n to verify its ability for measurements of neutron-induced reactions. In the beam test, a \(^{6}\)Li sample is mounted in the center of the cathode of the field cage. Figure 20 shows the typical track-display obtained in the beam test. For the track of triton, the Bragg distribution of dE/dx along the track is obviously identified, while the \(\alpha \)-particle has a much shorter track because of larger mass and higher charge. The time-of-flight (TOF) distribution of all triggered events is shown in Fig. 21. The peak located at the small TOF region is caused by the high-energy neutron events, leading to a gap of dead time of about 40 \(\upmu \)s. The distribution after the gap is mainly contributed from the reactions induced by neutrons on the \(^{6}\)Li sample. A particle identification (PID) between triton and \(\alpha \)-particle is shown in Fig. 22, verifying that the MTPC has a well PID ability which is limited if only the energy spectrum is obtained in the traditional method.

Fig. 20
figure 20

Typical tracks of triton (left) and \(\mathrm \alpha \)-particle

Currently, the finalized MTPC has been proposed and the new version of detector facility is under manufacturing. With this newly developed TPC detector system, a physical experiment will be conducted at the Back-n beamline in the nearly future.

Radiation-resistant semiconductor detector

Because of the excellent radiation resistance performance, wide-band gap semiconductor detectors are considered as an optimal option for silicon detectors. Among the wide-band gap semiconductor detectors, SiC and diamond detectors are widely studied for particle detection [43,44,45,46]. SiC and diamond detectors have the advantages of neutron and proton irradiation resistance, working normally at high temperatures [47,48,49]. In addition, due to the faster carrier drift speed and higher breakdown field strength, the rise time of output signals is faster than silicon detectors’. Thus, these detectors are suitable for fast measurement or time measurement [50].

4H-SiC detectors have been manufactured and tested at Back-n. The thickness of the substrate of the N-type 4H-SiC detector is 370\(~\upmu \)m, and the N-type 4H-SiC epitaxial material is produced by Cree Company. The epitaxial layer includes an N+ type 4H-SiC buffer layer with a thickness of about 500 nm and a 21\(~\upmu \)m-thick N-type 4H-SiC epitaxial layer with a doping concentration of \(1.5\times \mathrm {10^{14}}~\mathrm {cm^{-3}}\). A Ni/Au Schottky contact electrode with an area of 1\(~\mathrm {cm^{2}}\) was fabricated on the epitaxial layer, and an Al/Ti/Au ohmic contact electrode with an area of 1\(~\mathrm {cm^{2}}\) was fabricated on the substrate side.

The single-crystals diamond used at Back-n is high-quality single diamond crystals prepared by Zhengzhou University by microwave plasma chemical vapor deposition (MPCVD) and commercial detector-grade single diamond crystals produced by Element Six Company, with a size of 5.6\(\times \)5.5\(\times \)0.64\(~\mathrm {mm^{3}}\) and 4.5\(\times \)4.5\(\times \)0.5\(~\mathrm {mm^{3}}\), respectively. After multi-step cleaning, titanium and gold circular electrodes were evaporated on both sides of the single diamond crystal using thermal evaporation technology to form ohmic contacts and prevent metal oxidation, separately. Annealing at 650  \(^{\circ }\)C for 40 minutes ensures that a layer of Ti and C compounds is formed on the surface of the titanium and diamond, which increases the adhesion and reduces the potential barrier.

SiC and diamond detectors have been adopted to several cross section measurements and show good performance during experiments. Nevertheless, the area of diamond detectors and thickness of SiC detectors are still needed to be improved.

Fig. 21
figure 21

TOF distribution

Fig. 22
figure 22

PID of experimental data

Detectors for measuring reaction gammas

Radiative neutron capture cross section (\(\sigma _{n\gamma }\)) is of primary importance in studies of stellar nucleosynthesis, designs of advanced nuclear reactors, and applications of nuclear technology. Nowadays, mainly three kinds of detectors for \(\sigma _{n\gamma }\) measurement are used: total \(\gamma \)-ray absorption detectors, known as 4\(\pi \) \(BaF_{2}\) detector array [51], total energy detection system, such as \(C_{6}D_{6}\) [52], and high-resolution \(\gamma \)-ray detectors, such as HPGe detectors [53]. Since HPGe detectors are currently being designed and procured, only the first two are included in this section.

\(C_{6}D_{6}\) detection system

A detection system with four \(C_{6}D_{6}\) liquid scintillation detectors was chosen as the first \(\sigma _{n\gamma }\) measuring equipment at Back-n for its low neutron sensitivity, fast time response, and simple structure [54]. This \(C_{6}D_{6}\) detection system was installed at the center of ES#2 of Back-n, about 76 m away from the spallation target, shown in Fig. 23. The \(C_{6}D_{6}\) liquid scintillator was 127 mm in diameter and 76.2 mm in length, contained in a 1.5-mm-thick aluminum capsule and coupled with a photomultiplier tube (PMT). These \(C_{6}D_{6}\) detectors were placed upstream of the sample relative to the neutron beam, and the detector axis is at an angle of 125 degrees with respect to the neutron beam direction. The distance between the center of the front face of the detector and the sample center is about 150 mm. Anode signals delivered by the PMTs were recorded by the Back-n general-purpose Data Acquisition System (DAQ) [55], which digitizes the analog signals into full-waveform data with a sampling rate of 1 GS/s and a 12-bit resolution.

Fig. 23
figure 23

Photograph of the \(C_{6}D_{6}\) detection system at Back-n

To obtain high precision \(\sigma _{n\gamma }\), the weighting function (WF) of the \(C_{6}D_{6}\) detection system was calculated with the pulse height weighting technique (PHWT) [52, 54] and the experimental backgrounds were determined with dedicated measurements and Monte-Carlo simulations [56]. Besides, the resolution function was also studied to analyze the resonance parameters of \(^{232}\)Th and other nuclides [57]. With these studies, the \(\sigma _{n\gamma }\) in the energy region between 1 eV and 400 keV can be measured with this \(C_{6}D_{6}\) detection system [58, 59].

Gamma-ray total absorption facility

Gamma-ray total absorption facility (GTAF-II, which is the upgraded version of the earlier GTAF [60] according to the experiment of Back-n) has been constructed for accurate \(\sigma _{n,\gamma }\) measuring by prompt gamma method, which consisted of 40 barium fluoride detector units [61], shown in Fig. 24. The excited states in the compound nucleus that are populated by neutron capture can decay via many different gamma-ray cascades. The principle of detection is the sum energy of the cascade that corresponds to the binding energy of the captured neutron plus the kinetic energy of the captured neutron, it is usually about 6\(^{\sim }\)8 MeV. The BaF\(_2\) crystal shell with a thickness of 15 cm and an inner radius of 10 cm was subdivided into 12 pentagons and 28 hexagons, which covered 95.2\(\%\) of the solid angle. The overall time resolution (FWHM) of GTAF-II was 23.7 ns, and the detection efficiency of \(^{60}\)Co cascade gamma rays was 90\(\%\) [62]. The \(\sigma _{n,\gamma }\) experimental data of \(^{197}\)Au [63] and \(^{169}\)Tm were measured (neutron flight distance of 75.9 m). The position of resonance peak could be well consistent in comparison with the relevant data of ENDF evaluation database, which verified the reliability of GTAF-II and measurement technology. In the next step, high precision \(\sigma _{n,\gamma }\) of fission nuclides and radioactive nuclides could be obtained by deducting the background and improving the effect background ratio.

Fig. 24
figure 24

Photo of GTAF-II at Back-n

Fig. 25
figure 25

a Photograph and b schematic view of the imaging detector system

Detection systems for neutron resonance radiography

Thanks to the highest flux of the white neutron beam in the world, Back-n may have the best opportunity for the neutron resonance photography. The principle can be found in reference [64]. Two different systems are been developing tested at Back-n. A CMOS camera is a traditional image system, while the neutron-sensitive micro-channel-plate is still a novel technique.

Gated CMOS camera

A detector system with CMOS camera is constructed at Back-n white neutron source, which is mainly used in beam spot measurement, scintillator calibration, neutron imaging and other experiments. The system mainly consists of CMOS camera, neutron conversion scintillator and optical mirror, which are packaged in a light-shielding box, as shown in Fig. 25a.

The neutron conversion scintillator usually uses EJ426, which is still a novel technique for thermal neutrons with low sensitivity to gamma radiation [65]. The scintillator is a ZnS screen doped with \(^{6}\)LiF, and the thermal neutron detection efficiency of 0.5 mm thick is about 34\(\%\). As shown in Fig. 25b, the screen is placed in the center of the neutron beam, and its plane is perpendicular to the beam direction to detect neutrons by the well-known cross section of \(^{6}\textrm{Li} + \textrm{neutron} \xrightarrow {} ^{3}\textrm{H} + ^{4}\textrm{He} + 4.78\) MeV. The CMOS camera was purchased from Oxford Instrument Company, and its sensor size is 16.4 \(\times \) 14.0 mm\(^2\) with 2560 \(\times \) 2160 pixels. The typical spatial resolution of the camera is about 130 \(\upmu \)m. This camera has the ability to delay and select the time window, and the gate delay and width are adjustable from 0 to 10 s with the highest precision of 10 ps. The neutron energies are measured by the time-of-flight method. Therefore, this function of the camera can enable it to achieve energy-division photography and energy-resolved imaging on the Back-n.

Fig. 26
figure 26

Neutron profile distribution and grayscale information on x and y axis [1]

Fig. 27
figure 27

a Photograph and b neutron imaging of internal structures of the irregular marine condensate

Since March 2018, the camera system has carried out experiments such as standard beam spot measurement, scintillation screen calibration and neutron photography on the Back-n. A lot of research achievements have been obtained. As shown in Fig. 26, the \(\phi \)50 mm mode neutron profile distribution and grayscale information on x and y axis measured in the ES \(\#\)1 [66]. The beam spot distribution is independent of the neutron energy. For the neutrons with energy above 0.5 MeV, a more suitable plastic scintillator can be used instead of the ZnS(\(^{6}\)Li) screen. The standard beam spots in different modes of the Back-n are important beam parameters for the user experiments such as nuclear data measurement, radiation effect and neutron radiography.

For neutron radiography experiments, a remotely controlled FIXM sample platform is used to move a series of samples horizontally and vertically to save experimental time significantly. A rotating platform is used for neutron CT experiments. Neutron radiography is a method for investigating the inner structure of samples [67]. Compared with X-ray radiography, neutron radiography has a natural advantage in nuclide identification as neutron attenuation depends on the nuclear reaction between nucleus and neutron. Back-n has great potential in obtaining large-scale sample images due to its high flux and high-energy neutrons. Fig. 27a and b shows photograph and neutron imaging of internal structures of the irregular marine condensate, in which the shape of the ancient coins is clearly visible. The energy-selective photography of the CMOS camera enables it to perform nuclide resonance imaging measurements on the Back-n. In the resonance imaging, the neutrons with different energies are transmitted though the sample, then multiple radiographs are recorded by the camera with and without resonance neutrons. The nuclide components can be implied by processing the images [68]. Benefiting from the wide energy spectrum and high flux of the Back-n, various nuclides with cross section resonances in different energy regions are studied.

Neutron-sensitive micro-channel-plate

A neutron detector with energy and position resolution based on a \(^{10}\)B-doped micro-channel plate (B-MCP) is being under development on the Back-n. The B-MCP has high temporal resolution, spatial resolution, and high neutron detection efficiency. With the advantages of wide energy spectrum and high flux of Back-n, it is very suitable for neutron resonance imaging experiments. The B-MCP detector is generally composed of neutron-sensitive B-MCP group, readout anodes, vacuum chamber and voltage sources. Its main structure is shown in Fig. 28.

Fig. 28
figure 28

Schematic diagram of the structure of the B-MCP detector

Fig. 29
figure 29

The \(\phi \)30 mm beam profile in the \(\#\)ES2 measured by the B-MCP detector

Fig. 30
figure 30

Structure of full digital trigger mechanism

The neutrons react with the sensitive nuclide \(^{10}\)B in the B-MCP to produce secondary particles \(\alpha \) and \(^{7}\)Li, which excite secondary electrons on the inner wall of the B-MCP channel. The secondary electrons multiply in the channel under electric field to generate more secondary electrons and finally form an electron cloud at the exit of the channel to enhance the signal of the neutron event. To increase the collision probability between electrons and the channel and suppress ion feedback, the channel has an angle of about 5\(^{\circ }\)\(^{\sim }\) 10\(^{\circ }\) relative to the MCP surface normal, and generally, two MCP are used in combination with a V-shape of their channels. The \(^{10}\)B is one of the commonly neutron-sensitive nuclides, and its secondary particles \(\alpha \) and \(^{7}\)Li have a short range of only about 2\(^{\sim }\)3.5 \(\upmu \)m. Therefore, the secondary electrons are basically multiplied in several adjacent channels, and the spatial resolution of MCP can be better than 10 \(\upmu \)m. The transit time of secondary electrons in the MCP channel is at the ps level. The B-MCP can accept very high count rate with excellent time resolution. The detector system count rate limit and time resolution depend primarily on the electronics. The readout anodes of the B-MCP use an array of anode strips for the high flux neutron sources. The analytical spatial resolution of the charge center of gravity method can reach several tens of microns, which is sufficient for fast neutron imaging in most cases. B-MCP normally works at a vacuum of about 10\(^{-4}\) Pa \(^{\sim }\) 10\(^{-5}\) Pa. Therefore, the detector system needs to be sealed in a vacuum chamber. The \(^{10}\)B-doped B-MCP used in our experiments is about 10 mol\(\%\) content of the \(^{10}\)B nuclide. The test samples have a diameter of 33 mm and a thickness of 0.5 mm. We carried out beam spot measurements on Back-n using the B-MCP detector and studied the response of B-MCP to neutrons in different energy regions. As shown in Fig. 29, the measured \(\phi \)30 mm beam profile in the \(\#\)ES2 is clearly displayed, indicating that the development of the B-MCP detector is basically in line with expectations. The simulation study on signal response of the B-MCP is also carried out to provide a reference for the experimental analysis. The domestic development of \(^{10}\)B-doped B-MCP technology is being carried out in cooperating with the North Night Vision Technology Research Institute Co.Ltd, and it is difficult to dope \(^{10}\)B with high concentration consistence. Therefore, it is of great significance to study the properties of \(^{10}\)B-doped B-MCPs on Back-n.

Fig. 31
figure 31

Structure of readout electronics

Fig. 32
figure 32

Photography of electronics modules (from left to right: FDM, TCM, SCM and readout crate)

Fig. 33
figure 33

Hardware structure of DAQ system

Fig. 34
figure 34

GUI of run control and monitoring software

Common readout electronics

Good-performance electronics is a mandatory part of advanced spectrometers. Facing the challenge of high neutron flux, Back-n brings full digital trigger mechanism [69] and readout electronics [70, 71] with high performance. Figure 30 shows the principle of signal readout and data acquisition. On the top side, signal from neutron detector is fed into the signal condition module to generate proper signals which is compatible with the ultra high-speed digitizer. With the help of folding structure of analog digital converter, full digitized waveform of detector signal is obtained with very good magnitude and time resolution. The sampling rate can reach up to 1 GSas, while the resolution can be 12 bit. Based on the digitized waveform data, full digital trigger algorithm is proposed in Back-n as shown in Fig. 30. The L1 hardware digital algorithm is executed on FPGA (field programmable gate array). On each digitizer local FPGA, digitizing data stream is divided into two branches in parallel, one is fed into trigger match FIFO waiting for global trigger, and another one is fed into the sub-trigger processing module simultaneously. In the L1 hardware trigger structure, there is one master global trigger module, which receives all sub-trigger packet from all local trigger modules on each digitizer to generate the global trigger signal based on specific algorithm to indicate the valid good event occurs. This global trigger signal should be fanned out to each trigger match FIFO so that digitizer can readout the correct data corresponding to this good event. After being built, good event data are finally transmitted to the data acquisition server through ethernet. Besides the waveform measurement, in order to obtain the neutron energy precisely, the neutron TOF (time-of-flight) should be measured precisely in the electronics. The time-to-digital converter based on FPGA is adopted in readout electronics [72]. With experiment and evaluation, the accuracy of TOF can reach about 280 ps which is good for Back-n application.

To fulfill the full digital trigger algorithm efficiently, it is necessary to use industry advanced readout platform with the ability of excellent data transmitting throughput and system synchronization. Back-n adopts the PXIe platform to be the readout crate as shown in Fig. 31. The PXIe platform is based on high-speed serial PCIe bus, which can support ultra-high-speed of data bandwidth. Meanwhile, there are several differential buses with star structure on backplane (PXIE\(\_\)DSTARA, PXIE\(\_\)DSTARB and PXIE\(\_\)DSTARC), which can support for the global clock and trigger distributing and sub-trigger packets gathering. There are three different modules in the PXIe crate including TCM (trigger & clock module), SCM (signal condition module) and FDM (field digitizer module) as shown in Fig. 32. The FDM effective number of bits can be better than 9.2 bit among the frequency range of 398MHz with sampling rate of 1GSas, which guarantees that the readout electronics can meet the requirements of all Back-n spectrometers, especially the BaF\(_{2}\) spectrometer which has very fast signal edge.

DAQ

A data acquisition(DAQ) system is built for the general-purpose electronics and Back-n detectors. The hardware structure of DAQ system is shown in Fig. 33. PXI chassis controllers connect to a DAQ server through 1GbE/10GbE network. Three storage servers are deployed at the remote computer center and Gluster File System(GlusterFS) with excellent performance [73] is chosen for the management of storage resources. The storage system is close to the offline computing node, so that offline users are able to access the raw data more efficiently. Waveform data digitized by FDM board are readout by PXI chassis controllers and transferred to the DAQ server. The DAQ data flow software assembles the waveform packages into T0 Fragments(A T0 Fragment contains all events generated by a neutron bunch). T0 Fragments are fast processed in parallel for quality monitoring purposes. The whole The DAQ data flow runs on a single DAQ server with 56 CPU cores, data are processed in pipeline from readout to storage.

The run control and monitoring software is developed based on Django web framework. It communicates with the data flow software through Redis [74], in-memory data structure store. Control messages are sent throw Redis Pub/Sub interface and status parameters are updated periodically in Redis by the data flow software. Most online processing results are ROOT objects, which are also serialized to JSON string and published in Redis like status parameters. The JavaScript ROOT(JSROOT) library allows reading and displaying ROOT objects in an efficient way, and its rendering is now very d by ROOT [75]. So, the JSROOT library is used for visualization of online processing results in the Back-n monitoring software. The implementation of control and monitoring GUI of Back-n is shown in Fig. 34

Summary

In past 5 years, a preliminary detector system has been established. In order to ensure the common operation of the day-one experiments, these detection systems such as the fission chamber and the C\(_6\)D\(_6\) detectors adopt to the similar design of other white neutron beamlines. A update-designed common electrics and DAQ also supported these system while the beamline running.

In future, some more difficult experiments were proposed. Such as the MTPC, the GTAF-II and the B-MCP were developed to meet these requirements. Most of these detectors are at the forefront of detector research. With the completion of these detectors in the next few years, it is believed that Back-n will achieve excellent physical results in the research of small cross section and rare nuclear reaction physical events, the nucleosynthesis models of the astronomical nuclear physics and the archeology nondestructive detection, etc.